2000 360 engine- put in car or truck? What is needed?

No, the harness is mainly for the injectors and PCM. There is a problem with the LA intake manifolds fitting on the Magnum heads, though. I was told you can use the old style heads with the Magnum block. I was also told you can use the fuel injection with a "plug and play" aftermarket PCM.
You have to make provisions for your fuel pump. The new style Magnum has nowhere to bolt on a mechanical fuel pump. I don't know if the timing covers are interchangeable.

if you want to use a factory LA engine's intake you have to have the magnum heads re drilled for the bolt pattern

otherwise they make both a magnum 4 barrel intake, and a dual pattern LA and magnum 4 barrel intake

but if your putting a magnum engine in your vehicle why not go with the bonus of having EFI, its quite simple after you learn the components that make it run