If crank is 6.75 you would need a smaller dia WP pulley to spin it faster.
Or a larger dia crank pulley.
I would leave the crank pulley alone as it should be sized for the other accessories and just make the WP pulley smaller in dia to achieve a faster fan and pump speed.
5.5 to 6 would do it.
IIRC my 273 2bbl is 6.75 Crank And 6 WP stock but don't quote me.