Sizing for 64 Dart 270

Ok, how does this sound:

225/60r15 tires on 15*7 wheels in the rear. BF Goodrich 2 1/4” Whitewall

215/70r14 tires on 14*6 wheels in the front. BF Goodrich 2 1/4” Whitewall

The rear tires would be 25.6” diameter and the front would be 25.9” diameter. Difference of 6 revolutions per mile.

They’d be visually very similar looking from the side, roughly same total diameter, same size whitewall, but would be different widths. Hoping this can give me much better grip and help improve handling compared to the very thin 195mm wide tires I’ve got on all four corners currently.
You can. I used to run 15x7's on the back and 14's on the front when I had the black Rallys on the back. The Halibrand clone front wheels are skinny 15x4 1/2, the rears are 15x7. Front tires are 165 80 15 and the rears are 235 70 15. I have 255 60/15's on 15x7 rally's on mu swinger. I need to try them on my 66 someday just to see how they fit.