Is this LA360 XE268 cam kit deal good for my combo?

Stop thinking. That RPM range is merely a generic "guess" for advertisement purposes. That camshaft will pull well beyond 4500 RPM. Also, you need a better timing chain set if you expect to be able to zero in on the camshaft timing the way you need to. I would recommend one of the Cloyes billet sets with the nine way crank gear. Then you'll have something. Just DO what we're recommending. Turn the brain OFF and just DO IT. You'll be thankful, I promise. I wouldn't recommend something if I didn't think it would work. The cam card for that cam does not say to install it "STRAIGHT UP". If that's what you did, you are at least 4* retarded. Because of your low cylinder pressure, I recommend installing it down around a 106 ICL. That's 6* total advanced, instead of the recommended 4*. Once you get that done, then you can proceed to the ignition curve.
Ok. I must be stunod or something. First off, I didn't purchase my current crane cam but I thought dot to dot ( what I called straight up) was how mfg recommends installing the cam and it should perform as advertised barring any other engine mods. In the H-260-2 that would be 204/216 260/272 427/454, 112 lsa. Now don't some cams have " built in" advance? Are you saying dot to dot is 4 degrees retarded??
Second....I just bought a 3 key adjustable timing set for my magnum.
Can use on this LA. It's a double roller comp 3103. That would mean each key notch is 2 deg. It looks like I can only get 4 degrees max advance per comp. I'm at 112 and you recommended 108 so NG?? Remember, the LA is coming out summer of next year so doesn't need to be "optimal". Plus the car is most likely parked until spring.
Thanks.