Will this 71 a833 work in my 68?

Would it be “better” than a 68 with that ratio difference?
The 2.66 would give better acceleration in first gear, but it's not a massive difference. I had no worries in my '73 Challenger 340 with the 2.47 first. It certainly wasn't worth changing the transmission. It's about the same difference (in first gear only) as a 3.23 v. a 3.55 ring & pinion.